Review Notes-- chapter 17 Thermodynamics

            recommended problems: #23, 34, 40, 50, 62, 64, 66, 70, 88 (107)

Although the thermodynamics plays a role in a wide range of applications, the types of problems that might surface on the exam are quite limited.

            * As with almost everything we have been doing this semester, one critical element is a

                        balanced chemical equation for the reaction being considered. Without the

                        equation (or with an incorrectly balanced equation) nothing works correctly.

            * In this chapter, any temeprature used in a calculation must in in Kelvin

 

For the reaction you can compute DGo , DSo or DHo for the reaction

            from the standard thermodynamc tables (and these would cetrainly be provided)

            the superscript o means all species are in their standard state (1 atm, 1 M, or solid-liquid)

            since the table is at 25oC, the calculations are at 25oC

Typical Problem-- compute DGo , DSo or DHo for a reaction, or determine if a reaction

            is exothermic or if it is spontaneous (under standard conditions at 25 oC) Quite likely       

            to be given two of these (DGo , DSo or DHo) and asked to find the other or answer.

            DHo is the heat of reaction (negative if exothermic), typically 10-500 kJoule

            DGo is the free energy of the reaction (negative if reaction is spontaneous)  10-500 kJ

            DSo is the entropy change (positive if disorder increases)  typically a few Joule/deg

                        you can evaluate DGo from DGof values in the tables ..... or

                        you can evaluate  DHo and DSo and compbine  DGo=DHo - T DSo

                                    if you do this, be careful to avoid mixing kJoule and Joule

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There's a very useful link between DGo (25oC and Kequil (25oC)

            Kequil = exp (- DGo/RT)   or

            ln (Kequil) = - DGo / (RT)

                        so, from the thermodynamic tables, we can compute Kequil (first find DGo)

Typical problem: Given value for DGo (or for DSo and DHo) find Kequil. Or if Kequil = xxx, what

            is DGo for the reaction. Of course a spontaneous reaction has DGo <0 and so Kequil >1.

Note: the exp( ) function is the inverse of the ln ( ) function on your calculator

            usually [second] + [ln]  keys do this.

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We often want to know the value of DGo (or Kequil) at some other temperature.

            We can get a good estimate of DGo (another T)  by computing  DSo and DHo at 25oC

            and combining with a T other than 298 K. That value of DGo can be used to find Keq (T)

            or to determine if the reaction is spontaneous at this other temperature.

                        DGo= DHo - T DSo

Typical problem: if a reactions has DHo= xxx and DSo = yyy  at 25oC

            a. is the reaction spontaneous at 25oC?   b. at 450oC ?    c. at -140 oC ?

            d. at what temperature will a nonspontaneous reaction (25oC) beome spontaneous?

                        answer, when T = - DHo / DSo

            e. There are four cases (DHo ,  DSo are both negative), (DHo ,  DSo are both posative),

                        (DHo negative but   DSo postive) , and  (DHo positive,  DSo  negative) . When

                        could equation above (d) be used and why?

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The temperature dependence of Kequil was discussed in an earlier chapter

            a plot of ln (Kequil) vs 1/T (K) shows data as a straight line

            slope is - DHo / RT          (R=8.314, a value given on exam)

                        an exothermic graphic shows a + slope and Kequil decreases as T rises

                        an endothermic graphic shows a - slope and Kequil inccreases as T rises

                                    (that's what le Chatlier said earlier, remember?)

Typical problem: a table of Kequil is given at several temperatures

                                    find Kequil at another temeprature, find DHo for the reaction

                                    (may be easiest to calculate ln(K) and 1/T and plot the graph....

                                    on exam you may be given such data, already plotted)

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These rules / equations / ideas apply equally well to

            chemical reactions

            physical processes like evaporation (vapor pressure) or solubility (Ksp)

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Review Notes, Kinetics

there are really only a few major tasks (exam problems) in this chapter:

            find the order of the reaction (from data)

            find rate constant k (from data; you must know the order)

            how much remains (or is produced ) after __sec or how long until ___% has reacted ?

                        how to find and use half life data ?

            how will the rate of a reaction vary with temperature

                        or, what is Ea for the reaction?

Finding the order of a reaction

            Initial rate (slope of [reactant] vs. time )

                        how does it vary, from run to run, when you change initial concentrations of each?

            Rate when other species are in great excess (or are catalysts)

                        that is, when their concentration really doesn't vary during the run

            Subsequent half lives

            Fit data (conc of reactant vs. time ) to a graph  

                        if conc vs time is straight line-- zeroth order

                        if ln (conc) vs time is straight line-- first order

                        if 1/[conc] vs time is straight line -- second order

Finding the rate constant

            [rate of reaction]  / {concentrations }

            first order     k = ln(2) / t1/2           second order      k = 1 / ( [A]* t1/2 )

Finding out how much is left ... when

            ln (A/Ao) = - k*t          first

            1/[A] - 1/[Ao] = kt       second

            [A] = [Ao] - kt           zeroth

Energy of activation and temperature

            plot of ln (k) vs 1/T is straight line

            slope = -Ea / R